Assessing the corrosion protection of 8-hydroxyquinoline-cerium (III) complex for carbon steel in a NaCl solution
Author affiliations
DOI:
https://doi.org/10.15625/2525-2518/19391Keywords:
8-Hydroxyquinoline Complex, corrosion inhibitor, electrochemical impedance spectroscopy, cerium (III) ionsAbstract
In the present study, a complex between 8-hydroxyquinoline and cerium (III) (Ce-HQ) was synthesized in the presence of triethylamine. Afterwards, the complex was characterized by Field Emission Scanning Electron Microscopy (FESEM), Fourier-transform infrared spectroscopy (FTIR) and Thermo-Gravimetric Analysis (TGA). The inhibition efficiency of the Ce-HQ complex for the corrosion of carbon steel, evaluated by both Electrochemical Impedance Spectroscopy (EIS) and Potentiodynamic Polarization (PP) plots, reached 90 % after 2 h of immersion in a 0.01 M NaCl solution. Then, EIS measurements were carried out to evaluate the effect of the Ce-HQ complex, as inhibitive pigment, after incorporation in a waterborne epoxy coating applied over carbon steel plate. The total resistance (Rtotal) of the coated sample containing the Ce-HQ complex was higher (3.6 x 107 Ω cm2), after 35 days of exposure in a 0.5 M NaCl solution than the values obtained for the coating without Ce-HQ. The results showed that the EP/Ce-HQ coating provided not only corrosion protection by the Ce (III) ions and 8HQ release at the metal/coating interface, but also improved the barrier properties. This work proposed a new type of inhibitive pigments which can be used to develop effective coatings for corrosion protection.
Downloads
References
Dwivedi D., Lepková K., Becker T. - Carbon steel corrosion: a review of key surface properties and characterization methods, RSC Advances 7 (2017) 4580-4610. https://doi.org/10.1039/C6RA25094G
Aslam R., Mobin M., Zehra S., Aslam J. - A comprehensive review of corrosion inhibitors employed to mitigate stainless steel corrosion in different environments, J. Mol. Liq. 364 (2022) 119992. https://doi.org/10.1016/j.molliq.2022.119992
Hang T. T. X., Dung N. T., Truc T. A., Duong N. T., Truoc B. V., Vu P. G., Hoang T., Thanh D. T. M., Olivier M. G. - Effect of silane modified nano ZnO on UV degradation of polyurethane coatings. Prog. Org. Coat. 79 (2015) 68-74. https://doi.org/10.1016/ j.porgcoat.2014.11.008
Brenna A., Beretta S., Ormellese M. - AC Corrosion of Carbon Steel under Cathodic Protection Condition: Assessment, Criteria and Mechanism, A Review Materials 13 (9) (2020) 2158. https://doi.org/10.3390/ma13092158
Hang T. T. X., Truc T. A., Duong N. T., Pébère N., Olivier M. G. - Layered double hydroxides as containers of inhibitors in organic coatings for corrosion protection of carbon steel, Prog. Org. Coat. 74 (2012) 343-348. https://doi.org/10.1016/ j.porgcoat.2011.10.020
Truc T. A., Thuy T. T., Oanh V. K., Hang T. T. X., Nguyen A. S., Caussé N., Pébère N. - 8-hydroxyquinoline-modified clay incorporated in an epoxy coating for the corrosion protection of carbon steel, Surf. Interfaces 14 (2019) 26-33. https://doi.org/ 10.1016/j.surfin.2018.10.007
Salazar-Bravo P., Del Ángel-López D., Torres-Huerta A.M., Domínguez-Crespo M.A., Palma-Ramírez D., López-Oyama A.B. - Corrosion investigation of new hybrid organic/inorganic coatings for carbon steel substrates: Electrochemical and surface characterizations. Prog. Org. Coat. 135 (2019) 51-64. https://doi.org/10.1016/j.porgcoat.2019.05.038
Pepe A., Galliano P., Aparicio M., Durán A., Ceré S. - Sol-gel coatings on carbon steel: Electrochemical evaluation, Surf. Coat. Technol. 200 (2006) 3486-3491. https://doi.org/10.1016/j.surfcoat.2005.07.102
Thoume A., Elmakssoudi A., Left D.B., Benzbiria N., Benhiba F., Dakir M., Zahouily M., Zarrouk A., Azzi M., Zertoubi M. - Amino acid structure analog as a corrosion inhibitor of carbon steel in 0.5 M H2SO4: Electrochemical, synergistic effect and theoretical studies, Chem. Data Collect. 30 (2020) 100586. https://doi.org/10.1016/j.cdc.2020.100586
Badr G. E. - The role of some thiosemicarbazide derivatives as corrosion inhibitors for C-steel in acidic media, Corros. Sci. 51 (2009) 2529-2536. https://doi.org/10.1016/ j.corsci.2009.06.017
Chauhan D. S., Ansari K. R., Sorour A. A., Quraishi M. A., Lgaz H., Salghi R. - Thiosemicarbazide and thiocarbohydrazide functionalized chitosan as ecofriendly corrosion inhibitors for carbon steel in hydrochloric acid solution, Int. J. Biol. Macromol. 107 (2018) 1747-1757. https://doi.org/10.1016/j.ijbiomac.2017.10.050
Obot I. B., Ankah N. K., Sorour A. A., Gasem Z. M., Haruna K. - 8-Hydroxyquinoline as an alternative green and sustainable acidizing oilfield corrosion inhibitor. Sustainable Materials and Technologies 14 (2017) 1-10. https://doi.org/10.1016/j.susmat.2017.09.001
Mohammadloo H. E., Mirabedini S. M., Pezeshk-Fallah H. - Microencapsulation of quinoline and cerium based inhibitors for smart coating application: Anti-corrosion, morphology and adhesion study, Prog. Org. Coat. 137 (2019) 105339. https://doi.org/ 10.1016/j.porgcoat.2019.105339
Ivušić F., Lahodny-Šarc O., Ćurković H.O., Alar V. - Synergistic inhibition of carbon steel corrosion in seawater by cerium chloride and sodium gluconate, Corros. Sci. 98 (2015) 88-97. https://doi.org/10.1016/j.corsci.2015.05.017
Dastgheib A., Attar M.M., Zarebidaki A. - Evaluation of Corrosion Inhibition of Mild Steel in 3.5 wt% NaCl Solution by Cerium Nitrate. Met. Mater. Int. 26 (2019) 1634-1642. https://doi.org/10.1007/s12540-019-00432-x
Boudellioua H., Hamlaoui Y., Tifouti L., Pedraza F. - Effect of the temperature of cerium nitrate–NaCl solution on corrosion inhibition of mild steel. Corros. Mater. 71 (2020) 1300-1309. https://doi.org/10.1002/maco.201911472
Somers A. E., Hinton B. R. W., de Bruin-Dickason C., Deacon G. B., Junk P. C., Forsyth M. - New, environmentally friendly, rare earth carboxylate corrosion inhibitors for mild steel, Corros. Sci. 139 (2018) 430-437. https://doi.org/10.1016/j.corsci.2018.05.017
Dehghani A., Mostafatabar A. H., Ramezanzadeh B. - Synergistic anticorrosion effect of Brassica Hirta phytoconstituents and cerium ions on mild steel in saline media: Surface and electrochemical evaluations. Colloids Surf, A Physicochem. Eng. Asp. 656 (2023) 130503. https://doi.org/10.1016/j.colsurfa.2022.130503
Liu X., Zhang Y., Pan X., Wang Z. - Rare earth cerium-phenanthroline binary complex as a new corrosion inhibitor for carbon steel in acidic medium, Res. Chem. Intermed. 49 (2022) 1235-1257. https://doi.org/10.1007/s11164-022-04918-z
Hu Y., Cao X., Ma X., Pan J., Cai G., Zhang X., Dong Z. - A bifunctional epoxy coating doped by cerium (III)-8-hydroxyquinoline: Early self-reporting and stimuli-responsive inhibition on corrosion of Al substrate, Prog. Org. Coat. 182 (2023) 107616. https://doi.org/10.1016/j.porgcoat.2023.107616
Dehghani A., Ramezanzadeh B., Poshtiban F., Bahlakeh G. - Construction of a highly-effective/sustainable corrosion protective composite nanofilm based on Aminotris(methylphosphonic acid) and trivalent cerium ions on mild steel against chloride solution, Constr Build Mater. 261 (2020) 119838. https://doi.org/10.1016/j.conbuildmat. 2020.119838
Dehghani A., Bahlakeh G., Ramezanzadeh B., Mostafatabar A.H., Ramezanzadeh M. - Estimating the synergistic corrosion inhibition potency of (2-(3,4-)-3,5,7-trihydroxy-4H-chromen-4-one) and trivalent-cerium ions on mild steel in NaCl solution, Constr Build Mater. 261 (2020) 119923. https://doi.org/10.1016/j.conbuildmat.2020.119923
Abd El-Wahab Z.H. - Mixed ligand complexes of nickel(II) and cerium(III) ions with 4-(-3-methoxy-4-hydroxybenzylideneamino)-1, 3-dimethyl-2,6-pyrimidine-dione and some nitrogen/oxygen donor ligands, J. Coord. Chem. 61 (20) (2008) 3284-3396. https://doi.org/10.1080/00958970802039996
Liu C., Hou P., Qian B., Hu X. - Smart healable and reportable anticorrosion coating based on halloysite nanotubes carrying 8-hydroxyquinoline on steel, J. Ind. Eng. Chem. 118 (2023) 109-118. https://doi.org/10.1016/j.jiec.2022.10.050
Balaskas A. C., Kartsonakis I. A., Tziveleka L. A., Kordas G. C. - Improvement of anti-corrosive properties of epoxy-coated AA 2024-T3 with TiO2 nanocontainers loaded with 8-hydroxyquinoline, Prog. Org. Coat., 74 (2012) 418-426. https://doi.org/10.1016/ j.porgcoat.2012.01.005
Spengler E., Fragata F. L., Margarit I. C. P., Mattos O. R. - Corrosion protection of low toxicity paints, Prog. Org. Coat. 30 (1997) 51-57. https://doi.org/10.1016/S0300-9440(96)00668-6
Le Pen C., Lacabanne C., Pébère N. - Structure of waterborne coatings by electrochemical impedance spectroscopy and a thermostimulated current method: influence of fillers, Prog. Org. Coat. 39 (2000) 167-175. https://doi.org/10.1016/S0300-9440(00)00148-X
Le Pen C., Lacabanne C., Pébère N. - Characterisation of water-based coatings by electrochemical impedance spectroscopy, Prog. Org. Coat. 46 (2003) 77-83. https://doi.org/10.1016/S0300-9440(02)00213-8
Downloads
Published
How to Cite
Issue
Section
License
This work is licensed under a Creative Commons Attribution-ShareAlike 4.0 International License.
Vietnam Journal of Sciences and Technology (VJST) is an open access and peer-reviewed journal. All academic publications could be made free to read and downloaded for everyone. In addition, articles are published under term of the Creative Commons Attribution-ShareAlike 4.0 International (CC BY-SA) Licence which permits use, distribution and reproduction in any medium, provided the original work is properly cited & ShareAlike terms followed.
Copyright on any research article published in VJST is retained by the respective author(s), without restrictions. Authors grant VAST Journals System a license to publish the article and identify itself as the original publisher. Upon author(s) by giving permission to VJST either via VJST journal portal or other channel to publish their research work in VJST agrees to all the terms and conditions of https://creativecommons.org/licenses/by-sa/4.0/ License and terms & condition set by VJST.
Authors have the responsibility of to secure all necessary copyright permissions for the use of 3rd-party materials in their manuscript.