MODIFICATION OF GRAPHENE OXIDE BY CURCUMIN AND APPLICATION IN POLYURETHANE COATING
Keywords:graphene oxide, curcumin, corrosion protection, polyurethane coatings
Curcumin modified graphene oxide (GO-CR) was prepared using adsorption method and polyurethane (PU) coating containing 0.3 wt% GO-CR was prepared on carbon steel. Synthesized GO-CR was characterized by fourier transform infrared spectroscopy (FTIR), X-ray diffraction (XRD), scanning electron microscopy (SEM) and zeta potential measurement. Corrosion protection property of polyurethane coating containing GO-CR was evaluated and compared with blank polyurethane coating and coating containing GO by electrochemical impedance spectroscopy. The results showed that GO-CR has layer structure like GO with lower crystallinity. In GO-CR structure curcumin was attached on GO surface. The presence of curcumin on GO-CR surface provided corrosion inhibition action for PU coating and also improved the dispersion of GO in PU coating.
Yadav A., Kumar R., Choudhary H.K., Sahoo B. - Graphene-oxide coating for corrosion protection of iron particles in saline water, Carbon 40 (2018) 477-487.
Rehman Z.U., Raza M. A., Ghauri F. A., Kanwal R., Ahmad A., Inam A. - Graphene oxide coatings deposited on steel substrate using electrophoretic deposition and electrochemical evaluation of coatings in saline media, Key Engineering Materials 778 (2018) 111-117.
Ho C.Y., Huang S.M., Lee S.T., Chang Y.J. - Evaluation of synthesized graphene oxide as corrosion protection film coating on steel substrate by electrophoretic deposition, Applied Surface Science 477 (2019) 226-231.
Ramezanzadeh B., Bahlakeh G., Moghadam M.H.M., Miraftab R. - Impact of size-controlled p-phenylenediamine (PPDA)-functionalized graphene oxide nanosheets on the GO-PPDA/Epoxy anti-corrosion, interfacial interactions and mechanical properties enhancement: Experimental and quantum mechanics investigations, Chemical Engineering Journal 335 (2018) 737-755.
Sari M.G., Shamshiri M., Ramezanzadeh B. - Fabricating an epoxy composite coating with enhanced corrosion resistance through impregnation of functionalized graphene oxide-co-montmorillonite nanoplatelet, Corrosion Science 129 (2017) 38-53.
Parhizkar N., Ramezanzadeh B., Shahrabi T. - Corrosion protection and adhesion properties of the epoxy coating applied on the steel substrate pre-treated by a sol-gel based silane coating filled with amino and isocyanate silane functionalized graphene oxide nanosheets, Applied Surface Science 439 (2018) 45–59.
Jiang F., Zhao W., Wu Y., Wu Y., Liu G., Dong J., Zhou K. - A polyethyleneimine-grafted graphene oxide hybrid nanomaterial: Synthesis and anti-corrosion applications, Applied Surface Science 479 (2019) 963–973.
Saleh K.A., Mohammed M.K. - Inhibition and adsorption actions of nano curcumin for corrosion of carbon steel alloy in 3.5% NaCl Solution, International Journal of ChemTech Research 10 (3) (2017) 515-529.
Flores-Frias E.A., Barba V., Lucio-Garcia M.A., Lopez-Cecenes R., Porcayo-Calderon J., Gonzalez-Rodriguez J.G. - Use of curcuma and curcumin as a green corrosion inhibitors for carbon steel in sulfuric acid, Int. J. Electrochem. Sci., 14 (2019) 5026 – 5041.
Johnsirani V., Sathiyabama J., Rajendran S., Nagalakshmi R. - Curcumin dye as corrosion inhibitor for carbon steel in sea water, Chem Sci Trans. 2 (S1) (2013) S123-S128.
Nguyen T.D., Tran B. A., Vu K. O., Nguyen A.S., Trinh A.T., Pham G.V., To T.X.H., Phan M. V., Phan T.T. - Corrosion protection of carbon steel using hydrotalcite/graphene oxide nanohybrid, J. Coat. Technol. Res. 16 (2019) 585-595.
Esmaeili A., Entezari M.H. - Facile and fast synthesis of graphene oxide nanosheets via bath ultrasonic irradiation, J. Colloid Interface Sci. 432 (2014) 19–25.
Rohman A., Sudjadi D., Ramadhani D., Nugroho A. - Analysis of curcumin in curcuma longa and curcuma xanthorriza using FTIR spectroscopy and chemometrics, Research Journal of Medicinal Plant 9 (4) (2015) 179-186.
Bugli F., Cacaci M., Palmieri V., Di Santo R., Torelli R., Ciasca G., Di Vito M., Vitali A., Conti C., Sanguinetti M., De Spirito M., Papi M. - Curcumin-loaded graphene oxide flakes as an effective antibacterial system against methicillin-resistant Staphylococcus aureus, Interface Focus 8 (2018) 20170059.
Kittel J., Celati N., Keddam M., Takenouti H. - Influence of the coating–substrate interactions on the corrosion protection: characterisation by impedance spectroscopy of the inner and outer parts of a coating, Prog. Org. Coat. 46 (2003) 135-147
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